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Crystal structure and physical properties of the two stannides EuPdSn2 and YbPdSn2

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Fil: Sereni, J.G. Comisión Nacional de Energía Atómica. Instituto Balseiro. Departamento de Física. Laboratorio de Bajas Temperaturas; Argentina; Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Čurlík, I. University of Prešov, Faculty of Humanities and Natural Sciences; Eslovaquia
Fil: Giovannini, M. University of Genova, Department of Physics; Italia
Fil: Gastaldo, F. University of Genova, Department of Chemistry; Italia
Fil: Strydom, A.M. University of Johannesburg, Department of Physics, Highly Correlated Matter Research Group; Sudáfrica
Fil: Reiffers, M. University of Prešov, Faculty of Humanities and Natural Sciences; Eslovaquia; Slovak Academy of Science, Institute of Experimental Physics; Eslovaquia

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Centro Atómico Bariloche

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eng

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We report on synthesis, crystal structure and physical properties of the isotypic compounds YbPdSn2 and EuPdSn2 crystallizing in the MgCuAl2-type structure. In both stannides a divalent state of respective rare earth element was found from analysis of the magnetic susceptibilities. Whereas in YbPdSn2 only weak paramagnetic behaviour is observed, in EuPdSn2 a long-range magnetic phase transition occurs at 12.5 K with complex magnetic behaviour evidenced by magnetic susceptibity and specific heat measurements. Under the influence of magnetic field, the magnetic behaviour was found to evolve from an antiferromagnetic to a ferromagnetic state as a consequence of a re-arrangement of magnetic moments.

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I Čurlík et al 2018 J. Phys.: Condens. Matter 30 495802

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